EFFECT OF Cr ADDITION ON WETTABILITY AND REACTIVITY OF Ni-Cr ALLOY WITH MgO(100) SINGLE CRYSTALLINE SUBSTRATE

Natalia Sobczak 1,2 Rajiv Asthana 3 Robert Purgert 4 Rafal Nowak 1 Marta Homa 1 Jerzy Morgiel 5 Boguslaw Onderka 6
1Centre for High Temperature Studies, Foundry Research Institute, Krakow
2ZLG, Motor Transport Institute, Warsaw
3Manufacturing Engineering, University of Wisconsin-Stout, Menomonie, WI
4., Energy Industries of Ohio, Cleveland, OH
5Institute of Metallurgy and Materials Science, Polish Academy of Sciences, Krakow
6Non-Ferrous Alloys, AGH Technical University, Krakow
Magnesium oxide is widely used in the production of advanced refractory materials due to its specific thermophysical properties and high-temperature stability. It is widely used both as a base material or a sintering aid for the production of ceramic foundry appliances, crucibles and moulds for melting and casting of high-temperature Ni-based superalloys. Moreover, the same refractory materials are used also in the production of different appliances for various apparatuses used for testing thermodynamic and thermophysical properties of high-temeparture materials using container-assisted methods (e.g. in thermal analysis, calorimetry). Thus information on stability and reactivity of Ni-based alloys in contact with MgO-based ceramics is of both scientific and practical importance.

The sessile drop method coupled with contact heating procedure was applied for testing high temperature interaction of MgO(100) single crystalline substrates with liquid pure Ni, NiCr5 and NiCr10 alloy at 1500°C under flowing gas (Ar) of 900 mbar. After 15 min contact at the test temperature, the drop/substrate interface was opened by moving the drop to another position using a special manipulator. The solidified sessile drop samples were used for detailed structural characterization of interfaces using optical, SEM+EDS, HRTEM and scanning probe microscopy techniques.

Contrary to available data on wetting properties of Ni-based alloys on oxide-based ceramics, the NiCr10 alloy exhibits a good wetting and unusual wetting behavior on MgO single crystal: after reaching the lowest value of 68°, the contact angle increases up to 104° and wetting-dewetting phenomenon periodically repeats a few times during 15 min contact, both for the first and the second position of the drop on the substrate (after drop pushing to a new position).

The results obtained are analyzed from point of view of thermodynamic stability and reactivity in the NiCr-MgO system as well as of practical applications, particularly taking into account the reasons for the formation of such casting defects in Ni-superalloy castings as oxide-based inclusions and porosity.









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