IMF 2023

Invited
Visualization of switchable tribology of ferroelectrics using atomic force microscopy

Seongwoo Cho 1 Iaroslav Gaponenko 2,3 Kumara Cordero-Edwards 2 Jordi Barceló- Mercader 4 Irene Arias 4,5 Céline Lichtensteiger 2 Jiwon Yeom 1 Loïc Musy 2 Hyunji Kim 1 Gustau Catalan 6,7 Patrycja Paruch 2 Seungbum Hong 1,8
1Department of Materials of Science and Engineering, KAIST, Daejeon, South Korea
2Department of Quantum Matter Physics, University of Geneva, Geneva, Switzerland
3G.W. Woodruff School of Mechanical Engineering, Georgia Institute of Technology, Atlanta, USA
4Laboratori de Càlcul Numèric, Universitat Politècnica de Catalunya, Barcelona, Spain
5(CIMNE), Centre Internacional de Mètodes Numèrics en Enginyeria, Barcelona, Spain
6Institut Català de Nanociència i Nanotecnologia (ICN2), Campus Universitat Autonoma de Barcelona, Barcelona, Spain
7(ICREA), Institució Catalana de Recerca i Estudis Avançats, Barcelona, Spain
8KAIST Institute for NanoCentury (KINC), KAIST, Daejeon, South Korea

Here, we visualize the switchable friction and wear behavior of ferroelectrics using a nanoscale scanning probe. The down domains have lower friction coefficient than up domains, of which asymmetry is enabled by flexoelectrically coupled polarization in the up and down domains under a sufficiently high contact force. Using this switchable tribology and multi-pass patterning with a domain-based dynamic smart mask, we demonstrate three-dimensional nanostructuring exploiting the asymmetric wear rates of up and down domains, which can, furthermore, be scaled up to technologically relevant (mm-cm) size.









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