Chirality is at the origin of life and is ubiquitous in nature. An object is deemed chiral if it is non-superimposable with its own mirror image, which is then relates to a particular way a circularly polarized light interacts with such object – known as circular dichroism (CD), the differential absorption of left- and right-circularly polarized light. The conventional understanding of chiroptical effects in biology, chemistry and physics, results from an internal chiral structure or, in a special two-dimensional case, the extrinsic symmetry breaking under asymmetric illumination. Here we show that CD is possible with simple symmetric optical nanoantennas at symmetric illumination, that is – at normal incidence of light. We demonstrate that the phase lag between two electromagnetic dipole-like modes, in principle, suffice to produce far-field chiroptical response in achiral structure. This has been exemplified both is experimentally and theoretically with the all-visible spectrum archetypical optical nanoantennas – symmetric nanoellipses and nanodimers, forming large-scale metasurfaces. The simplicity and generality of this finding reveal a whole new significance of the electromagnetic design and complex media engineering at a nanoscale with potential far-reaching implications for optics in biology, chemistry and materials science.
addis@chalmers.se